Ex Parte Mercx et alDownload PDFPatent Trial and Appeal BoardFeb 28, 201711034520 (P.T.A.B. Feb. 28, 2017) Copy Citation United States Patent and Trademark Office UNITED STATES DEPARTMENT OF COMMERCE United States Patent and Trademark Office Address: COMMISSIONER FOR PATENTS P.O.Box 1450 Alexandria, Virginia 22313-1450 www.uspto.gov APPLICATION NO. FILING DATE FIRST NAMED INVENTOR ATTORNEY DOCKET NO. CONFIRMATION NO. 11/034,520 01/12/2005 Franciscus Petrus Maria Mercx 150701-2-US-NP 8442 52674 7590 03/02/2017 Raker & Hostetler T T P EXAMINER 1170 Peachtree Street NE KOLLIAS, ALEXANDER C Suite 2400 Atlanta, GA 30309-7676 ART UNIT PAPER NUMBER 1767 NOTIFICATION DATE DELIVERY MODE 03/02/2017 ELECTRONIC Please find below and/or attached an Office communication concerning this application or proceeding. The time period for reply, if any, is set in the attached communication. Notice of the Office communication was sent electronically on above-indicated "Notification Date" to the following e-mail address(es): eofficemonitor@bakerlaw.com PTOL-90A (Rev. 04/07) UNITED STATES PATENT AND TRADEMARK OFFICE BEFORE THE PATENT TRIAL AND APPEAL BOARD Ex parte FRANCISCUS PETRUS MARIA MERCX, CARLO PEREGO, and ROBERT PUYENBROEK Appeal 2015-002326 Application 11/034,5201 Technology Center 1700 Before ADRIENE LEPIANE HANLON, MICHAEL P. COLAIANNI, and CHRISTOPHER L. OGDEN, Administrative Patent Judges. OGDEN, Administrative Patent Judge. DECISION ON APPEAL Appellants appeal under 35 U.S.C. § 134(a) from the Examiner’s decision2 finally rejecting claims 13, 15, and 173 in the above-identified application. A hearing was held on February 14, 2017. We have jurisdiction pursuant to 35 U.S.C. § 6(b). We AFFIRM. 1 Appellants identify SABIC Global Technologies BV. Appeal Br. 1, Sept. 25, 2014. 2 Final Office Action, Mar. 31, 2014 [hereinafter Action]; Examiner’s Answer, Nov. 6, 2014 [hereinafter Answer]. 3 Appeal Br. 1. The Action also rejected claims 1—4, 6, 8, 9, 11, 14, 16, and 18—23. See Action 1. These claims were canceled prior to the appeal. See Advisory Action 2, July 10, 2014 (entering amendment canceling claims). Appeal 2015-002326 Application 11/034,520 BACKGROUND Appellants’ invention relates to “a fiber reinforced flame-retardant polyamide composition having a combination of good flame retardant properties, good electrical performance such as arc tracking resistance, and good mechanical properties.” Spec. 1 5. According to Franciscus Petrus Maria Mercx, one of the listed inventors, polyamide resins provide outstanding heat resistance and mold workability, but show poor flame resistance, making it necessary to add flame retardants when used in electrical applications. See Mercx Decl. 12, Mar. 17, 2014; accord Spec. 12. It was known in the art to reinforce polyamide materials with glass, but according to Mr. Mercx, these known materials were unable to meet all industry requirements, such as a VO rating under the UL-94 flammability standard. See Marcx Decl. 112; accord Spec. 13. During experimentation, Mr. Mercx states that the inventors initially found that “it was impossible to extrude a strand of polyamide containing between 35% and 60% by weight of glass fibers and a flame retardant additive.” Id. H 14—15. According to Mr. Mercx, the mixture “cannot be uniformly mixed and extruded into a uniform strand. The presence of such a large amount of filler causes seizure of the extruder and thus prevents production of the composition.” Id. 119. However, the inventors claim to have solved this problem by discovering a flame-retardant polyamide composition, with 35 wt.% or more of glass filler, that can be extruded. See id. 116. Independent claim 13, the sole independent claim on appeal, is representative of this composition: 2 Appeal 2015-002326 Application 11/034,520 13. A flame-retardant polyamide composition, comprising: 30 to 65% by weight nylon-6, nylon-6,6, or a combination thereof; 10 to about 40% by weight of a halogen-free flame retardant system comprising i) a metal phosphinate of the formula (1) or the metal diphosphinate salt of the formula (11) 0 r o O 1 , II R1—P---- O 1 Mx II , IIO--- P----R3—P----O 1 1 1 R2 m R1 R2 (I) (II) wherein R1 and R2 are each independently hydrogen, a linear or branched C1-C6 alkyl radical, or aryl radical; R3 is a linear or branched Ci-Cio alkylene, arylene, aklylarylene, or arylalkylene radical; M is calcium, aluminum, magnesium, strontium, barium, or zinc; m is 1, 2, or 3; n is 1 or 3; and x is 1 or 2; and ii) at least one nitrogen compound selected from the group consisting of benzoguanine compounds, terephthalic ester compounds of tris(hydroxyalkyl)isocyanurate, allantoin compounds, glycoluril compounds, melamine cyanurate, melamine phosphate compounds, dimelamine phosphate compounds, melamine pyrophosphate compounds, melem, melam, and combinations thereof; and 35 to 60% by weight percent glass fiber wherein all the amounts are based upon the total weight of components; wherein a molded sample of the composition exhibits a rating of VO according to UL-94 at 1.6 millimeters thickness; wherein the composition exhibits a tensile modulus of at least about 10.5 GPA measured according to ISO Standard 52711 as measured on a sample having a thickness of 4.0 millimeters; and wherein the composition exhibits a comparative tracking index measured according to International Electrotechnical Commission standard 1EC-60112/3rd of greater than about 400 Volts. 3 Appeal 2015-002326 Application 11/034,520 Appeal Br. 16. Claims 15 and 17 depend from claim 13. Id. at 17. The Examiner maintains the following grounds of rejection4: 1. Claims 13 and 17 are rejected under 35 U.S.C. § 103(a) as being unpatentable over Steenbakkers-Menting.5 See Action 4, 7—8. 2. Claim 15 is rejected under 35 U.S.C. § 103(a) as being unpatentable over Steenbakkers-Menting, in view of Koning.6 See Action 12-14. In the Appeal Brief, Appellants argue claims 13 and 17 as a group, see Appeal Br. 5—15, and rely on the same arguments regarding dependent claim 15, see id. at 15. Therefore, consistent with 37 C.F.R. § 41.37(c)(l)(iv) (2016), we limit our discussion to claim 13, and claims 15 and 17 stand or fall with claim 13. DISCUSSION The Examiner finds that Steenbakkers-Menting discloses a polyamide composition comprising 10-95 wt.% of a polyamide, 5^40 wt.% of a halogen-free flame retardant system comprising a metal phosphinate or disphosphinate salt and a nitrogen compound, and 0—50 wt.% of glass fiber. Action 7. While claim 13 requires that the polyamide is either nylon-6 or nylon-6,6, see Appeal Br. 16, the Examiner finds that Steenbakkers-Menting 4 The Examiner has withdrawn an additional rejection of claims 13, 15, and 17 under 35 U.S.C. § 112, second paragraph. See Answer 2. 5 Steenbakkers-Menting et al., Patent Application Pub. No. US 2004/0021135 Al (published Feb. 5, 2004). 6 Koning et al., Patent Application Pub. No. EP 0 374 988 Al (published June 27, 1990). 4 Appeal 2015-002326 Application 11/034,520 teaches a preference for nylon-6, nylon-6,6, or nylon-4,6,7 two of the three of which are among the choices available for the polyamide component in claim 13. See Answer 13 (citing Steenbakkers-Menting |378). The Examiner also finds that Steenbakkers-Menting discloses a preferred flame retardant component comprising a genus of metal phosphinate or diphosphinate salts that is a subset of the genus defined in claim 13, part (i). Id. at 12—13 (citing Steenbakkers-Menting 123). In addition, the Examiner finds that Steenbakkers-Menting teaches that the flame retardant component comprises four preferred nitrogen compounds, two of which (melem and melam), are among the choices available for the nitrogen compound in claim 13, part (ii). Id. at 13 (citing Steenbakkers-Menting 122). Thus, the Examiner finds that Steenbakkers-Menting teaches the composition of claim 13, in concentration ranges that overlap the ranges set forth in the claim. See Action 7. The Examiner recognizes that Steenbakkers-Menting does not explicitly disclose the property limitations (rating under the UL-94 standard, tensile modulus, and comparative tracking index) set forth in the claim’s final three paragraphs. Nonetheless, due to overlap of the preferred components disclosed in Steenbakkers-Menting, the Examiner concludes that a prima facie of obviousness has been established. See id. at 8 (citing In re Best, 562 F.2d 1252, 1255 (CCPA 1977)). 7 Steenbakkers-Menting refers to nylon-6, nylon-6,6, and nylon-4,6 as PA (polyamide) 6, PA 66, and PA 46, respectively. See Steenbakkers- Menting 137. 8 The Examiner cites paragraph 36 of Steenbakkers-Menting, but evidently intended to cite the next paragraph, which states, “Preferably polyamide 6, PA 66 or PA 46 are chosen. . . . The polyamide in the flame retardant polyamide composition according to the invention is in particular polyamide 6.” 5 Appeal 2015-002326 Application 11/034,520 According to the Examiner, the claimed properties are inherent in the teachings of Steenbakkers-Menting. See id.', see also PAR Pharm., Inc. v. TWIPharm., Inc., 773 F.3d 1186, 1195 (Fed. Cir. 2014) (concept of inherency when applied to obviousness “is present only when the limitation at issue is the ‘natural result’ of the combination of prior art elements”). The Examiner also determines that Steenbakkers-Menting teaches a finite number of identified, predictable solutions (the preferred embodiments), and that the invention is obvious because a person of ordinary skill in the art would have had a reasonable expectation of success in choosing a composition within the scope of claim 13. See Answer 14 (citing MPEP §2143). Appellants argue that the Examiner’s rejection is legally and factually erroneous, and that the weight of evidence favors patentability. We address Appellants’ arguments as follows: 1. The Examiner s Prima Facie Case Appellants argue that the Examiner has not established a prima facie case of obviousness. First, Appellants argue that Steenbakkers-Menting teaches a broad genus of compounds, and that to arrive at compounds within the scope of claim 13 would require “fortuitous picking and choosing based upon impermissible hindsight.” Reply Br. 2. According to Appellants, “the fact that a claimed species or subgenus is encompassed by a prior art genus is not sufficient by itself to establish a prima facie case of obviousness.” Appeal Br. 5 (citing In re Baird, 16 F.3d 380, 382 (Fed. Cir. 1994); In re Jones, 958 F.2d 347, 350 (Fed. Cir. 1992); MPEP § 2144.08 II); see also Reply Br. 3. 6 Appeal 2015-002326 Application 11/034,520 This argument does not persuade us that the Examiner reversibly erred in rejecting claim 13. The mere fact that Steenbakkers-Menting discloses a multitude of effective combinations does not render any particular combination less obvious. This is especially true in this case where the claimed composition is used for the identical purpose taught by the prior art (i.e., flame retardant polyamide compositions). Merck & Co., Inc. v. Biocraft Labs., Inc., 874 F.2d 804, 807 (Fed. Cir. 1989). Moreover, while Steenbakkers-Menting discloses a broad genus of compounds, only a few of which are within the scope of claim 13, the reference provides teachings that would have guided a person of ordinary skill in the art toward a mixture of components within the scope of Appellants’ claimed invention. For example, while Steenbakkers-Menting discloses many possible polyamide compounds, the reference teaches a preference for three of them, including nylon-6 and nylon-6,6. See Steenbakkers-Menting 137. We also note that Steenbakkers-Menting teaches that the most preferred polyamide is nylon-6. See id. Steenbakkers- Menting also teaches the metal phosphinate or metal diphosphinate salts of formulas (I) and (II) of claim 13, see id. H 6—13, and teaches that preferably, “R1 and R2 are a linear or branched C1-C6 alkyl radical or phenyl” because this results in better stability of the compound. Id. 123. The reference teaches that M is preferably “Ca, A1 or Zn,” because “less polymer degradation takes place in the polyamide composition during preparation and processing.” Id. 124. Steenbakkers-Menting teaches a preference for four nitrogen compounds corresponding to component (ii) in claim 13, see 7 Appeal 2015-002326 Application 11/034,520 id. 122, and two of these, melam and melem, are among the choices listed in claim 13, see Appeal Br. 16.9 Thus, a person of ordinary skill in the art, following the preferences taught by Steenbakkers-Menting, would have needed to make only a very few choices from among the preferred embodiments to arrive at the chemical structure of the specific components set forth in claim 13. The facts on this record are substantially different from In re Baird, where the disclosed generic formula encompassed more than 100 million different chemical structures, only one of which was within the scope of the claim at issue. See 16 F.3d at 382. Likewise, in In re Jones, the prior art reference disclosed a “potentially infinite genus” of compounds, whereas the claim was directed to a specific compound. See 958 F.2d at 350. The Examiner’s determination that the combination of chemical components in claim 13 would have been obvious in view of Steenbakkers-Menting is rationally based on the teachings and preferences expressed by the reference, and not on fortuitous picking and choosing based on impermissible hindsight. The Examiner’s prima facie case of obviousness is also based on the fact that the concentration ranges for the components disclosed by Steenbakkers-Menting overlap the ranges specified in claim 13. The range of 10-95% of polyamide, see Steenbakkers-Menting 130, overlaps the range of 30-65% in claim 13. The range of 5 40% flame retardant and the preferred ranges of 10—35% and 15—30%, see Steenbakkers-Menting || 32, 36, overlap the range of 10-40% in claim 13. The range of 0—50% glass 9 Of the four preferred choices, however, the most preferred compound, melamine, is not listed among the permissible nitrogen compounds in claim 13. See Appeal Br. 16. We do not find this dispositive, given that Steenbakkers-Menting still expresses a preference for melem and melam. 8 Appeal 2015-002326 Application 11/034,520 fiber and the preferable ranges of 10-40% and 20-35%, see Steenbakkers- Menting H 31, 35, 38, overlap or touch the range of 35—60% glass fiber in claim 13. Typically, a prima facie case of obviousness exists when the ranges of a claimed composition overlap the ranges disclosed in the prior art. In re Peterson, 315 F.3d 1325, 1329 (Fed. Cir. 2003). This is particularly true here, where not only the broader range of 0-50% glass overlaps that of claim 13, but the narrower preferred range of 10-40% and the most preferred range of 20-35%, which touches the range of glass fiber content in claim 13 at its lower end. Appellants argue that despite the overlapping ranges for glass fiber content, Steenbakkers-Menting teaches away from the range of 35—60% because all the working example in Steenbakkers-Menting, which represent the reference’s only specific guidance, include only 25% glass fiber; thus, a person of ordinary skill in the art would have been led on a path divergent from the upper end of the ranges otherwise disclosed by the reference. See Appeal Br. 6—7; Reply Br. 6 (citing Teva Pharms. USA, Inc. v. Sandoz, Inc., 723 F.3d 1363, 1372 (Fed. Cir. 2013)). Teaching away is a question of fact, see In re Harris, 409 F.3d 1339, 1341 (Fed. Cir. 2005). Based on the facts of this record, including Steenbakkers-Menting as a whole,10 we do not find Appellants’ argument persuasive of reversible error. Although Steenbakkers-Menting does not describe any specific, working examples in which the glass fiber content is within the range of 35—60%, Appellants have not pointed to evidence 10 See In re Fracalossi, 681 F.2d 792, 794 n.l (CCPA 1982) (“It is axiomatic that a reference must be considered in its entirety, and it is well established that the disclosure of a reference is not limited to specific working examples contained therein.”). 9 Appeal 2015-002326 Application 11/034,520 persuasively showing Steenbakkers-Menting to “criticize, discredit, or otherwise discourage the solution” in claim 13. In re Fulton, 391 F.3d 1195, 1201 (Fed. Cir. 2004). To the contrary, we read the reference as encouraging the use of fiber content of up to at least 35%, which is the upper bound of the most preferred embodiment. See Steenbakkers-Menting 138. Steenbakkers-Menting also teaches that using glass fiber in a range extending up to 40% has advantages over the prior art, including “a V-0 rating according to UL 94” and “good mechanical properties, particularly a high breaking strength and a high elongation at break.” Id. 135. The Federal Circuit’s holding in Teva v. Sandoz does not require a different conclusion. In that case, the prior art reference taught that molecular weights below a certain level were “ineffective for treating multiple sclerosis,” and therefore the reference taught away from the use of lower molecular weights. See 723 F.3d at 1372. By contrast, Appellants have not directed our attention to any teaching in Steenbakkers-Menting that glass content of 35% or higher would have been ineffective or inoperable. To the contrary, Steenbakkers-Menting teaches a preference for glass content in a range extending up to 35% and as high as 40%. Appellants also argue that “the Examiner has misapprehended and thus, misapplied the principles of In re Best” in shifting the burden to Appellants to show that the compositions disclosed in Steenbakkers-Menting do not necessarily have the properties required by claim 13. See Appeal Br. 7. According to Appellants, the Examiner has failed to provide the required factual and technical analysis, and has not taken into consideration evidence from the record (in particular, Table 4 of the Specification); thus, a factual basis for burden shifting has not been established. See id. at 7—8. Appellants 10 Appeal 2015-002326 Application 11/034,520 also argue that the scope of compounds disclosed by Steenbakkers-Menting is much broader than the scope of claim 13, and the evidence shows that only a small subset of these compounds have the properties set forth in claim 13. See id. at 11—12. We do not find these arguments persuasive of reversible error. As discussed above, a person of ordinary skill in the art, following the preferences taught in Steenbakkers-Menting, would have been led to specific components within the scope of claim 13, in amounts that substantially overlap the scope of claim 13. Therefore, the Examiner has established a prima facie case of obviousness, and the burden has shifted to Appellants to produce evidence of non-inherency. See Best, 562 F.2d at 1255. To rebut the Examiner’s prima facie case, Appellants must point to evidence that the properties of claim 13 are not necessarily present or “the natural result of the combination of elements explicitly disclosed by the prior art.” PAR Pharm., 773 F.3d at 1196; see also Best, 562 F.2d at 1255. We have considered Appellants’ proposed evidence against inherency on this record, but do not find this evidence persuasive or sufficient to rebut the Examiner’s finding of inherency. In particular, Appellants point to Table 4 of the Specification, which is reproduced below: 11 Appeal 2015-002326 Application 11/034,520 Table 4. Components 17 IS 19 20 21 22 1 23 24 25 PA 6 2(4RV 34.70 29.70 24.70 19.70 35.95 34.70 32.20 28.45 27.20 PA66 2.4RV 34.70 29.70 24.70 19.70 7*} 94 34.70 12.20 28.45 27.20 Glass Fiber 15.00 25.00 35.00 45.00 25 00 25,66 25.00 25.00 25.66 Component A 15.00 15.00 15,00 15.00 2,50 5.00 17.50 20.00 AOl 0.20 " 0.20 0.20 0.20 0.20 0.20 0,20 0.20 0.20 A 02 6. is 0.15 6.15 0.15 0.15 i 0.! 5 1 6.15 0.15 6.15 Mold release 0,25 6.25 0.25 0,25 0.25 0.25 0,25 0.25 6.25 Properties. \ Tensile Modulus (GPa) 6,8 9.4 12,2 14,1 S.9 8,4 8.9 i 9.5 i 9,7 Tensile Strength (MPa) 112.0 140.0 166,5 189.3 161,2 153.5 155.0 .............. 138,0 125.0 Iscod notched impact {KJ/mb 7.4 9,5 . n.2 12.4 8.7 9,2 8.6 j 9.0 j 7.5 I 1 CT1('volts) 600 0 600 600 600 600 600 600 600 GWFi 96(PC (Si 1,0mm pass pass pass pass fail pass pass pass pass UL class ijSj Q.Smm V2 V2 VO VO V2 V2 V2 VO VO UL class @ 1 6mm VO VO VO VO V2 V2 VQ vo Table 4 shows various properties, including compositions of components and tensile modulus, for various materials designated as Examples 17—25. Appellants argue that only Examples 19 and 20 possess a tensile modulus of at least 10.5 GPa as required by claim 13. Appeal Br. 8. However, the fact that Examples 17, 18, and 21—25 are shown to have a lower tensile modulus is not persuasive evidence of non-inherency. These comparative examples are already outside the scope of claim 13 in terms of their glass fiber composition, so their tensile modulus is not relevant to the question of whether or not compounds disclosed by Steenbakkers-Menting with 35—50% by weight glass fiber would inherently possess a tensile modulus within the scope of claim 13. Moreover, both examples 19 and 20 have glass fiber compositions within the broad range of 0-50% disclosed by Steenbakkers- Menting, and Example 19 is within the preferred range of 10-40%. See id.', 12 Appeal 2015-002326 Application 11/034,520 see Answer 7—8 (finding that Example 19 is taught by Steenbakkers-Menting and necessarily possesses the properties of claim 13). Thus, Table 4 does not constitute evidence that a tensile strength of 10.5 GPa is not the natural result of a combination of elements taught by the preferences of Steenbakkers-Menting.11 In addition, other evidence on this record supports the Examiner’s finding of inherency. Regarding the requirement in claim 13 that “a molded sample of the composition exhibits a rating of VO according to UL-94 at 1.6 millimeters thickness,” see Appeal Br. 16, we note that Steenbakkers- Menting teaches that the disclosed flame retardant polyamide composition containing 10-40% glass fiber exhibits “a V-0 rating according to UL 94.” Steenbakkers-Menting 135. Regarding the requirement in claim 13 that “the composition exhibits a tensile modulus of at least about 10.5 GPA measured according to ISO Standard 5271112 as measured on a sample having a thickness of 4.0 millimeters,” see Appeal Br. 17, Steenbakkers- Menting also provides evidence that such a composition “shows good 11 In addition to finding that Table 4 of the Specification is insufficient evidence of non-inherency, the Examiner alternatively finds that each of the compositions within the scope of claim 13 “necessarily must possess the properties recited in the claims and therefore it is the Examiner’s position that the properties flow as a consequence of the claimed composition.” Answer 4. In other words, the Examiner determines that the property limitations of claim 13 are non-limiting. See id.', see also Appeal Br. 12 (arguing against this determination); Reply Br. 3^4. Because we find that Steenbakkers-Menting teaches a preferred set of compositions for which the properties of claim 13 are a natural result, we do not address the Examiner’s alternative finding as to the scope of claim 13. 12 While the claim refers to “ISO Standard 52711,” the Specification refers to “ISO Standard 527/1,” Spec. 42, 47, which appears to indicate that claim 13 has a typographical error. 13 Appeal 2015-002326 Application 11/034,520 mechanical properties, particularly a high breaking strength and a high elongation at break, as measured for example in a tensile test according to ISO 527-1.” Steenbakkers-Menting 135. We have considered Appellants’ argument that “the Examiner cites to no evidence that every possible composition that is described within the vast genus of Steenbakkers necessarily has the properties of the compositions set forth in claim 13.” Appeal Br. 11—12. However, we find this argument unpersuasive of reversible error. Inherency does not require that every possible composition taught by a prior art reference have the claimed properties. Inherency is established if the claimed properties are “the natural result of the combination of elements explicitly disclosed by the prior art.” PAR Pharm., 773 F.3d at 1196. As discussed above, Steenbakkers-Menting teaches at least some combinations of elements that fall within the scope of the compositional limitations of claim 13, and Appellants have not pointed to any persuasive factual evidence that Steenbakkers-Menting would not have led a person of ordinary skill in the art to compositions for which the claimed properties are a natural result. 2. Unexpected Results Appellants point to evidence in the Specification, and in the Mercx Declaration, that the composition of claim 13 is nonobvious because it exhibits unexpected results. See Appeal Br. 3—4, 7—8. In the Specification, Appellants point to Table 4, comparing Examples 19 and 20 with comparative Examples 17, 18, and 21—25, as “a factual basis to reasonably conclude that the compositions of claim 13 are non-obvious over the exemplified compositions of Steenbakkers[-Menting].” Appeal Br. 8. According to Appellants, Table 4 shows “compositions within the scope of 14 Appeal 2015-002326 Application 11/034,520 claim 13 that contain at least 35% glass fibers possess an unexpected increase in tensile modulus than compositions having less glass fiber.” Id. at 9. For us to find unexpected results, the record must show “(1) that there actually is a difference between the results obtained through the claimed invention and those of the prior art; and (2) that the difference actually obtained would not have been expected by one skilled in the art at the time of invention.” In re Freeman, 474 F.2d 1318, 1324 (CCPA 1973) (citation omitted). Although Examples 19 and 20 show an increased tensile modulus, Appellants do not point to persuasive factual evidence that the increased tensile modulus would have been unexpected to one of ordinary skill in the art as compared to the other examples that have less glass fiber content. To that end, Steenbakkers-Menting teaches that glass fiber content of from 10 to 40% provides good mechanical properties. See Steenbakkers-Menting 1131,35,38. In addition, establishing unexpected results requires that the comparative examples are truly comparative, and that the cause and effect relationship sought to be proven is not “lost... in the welter of unfixed variables.” In re Dunn, 349 F.2d 433, 439 (CCPA 1965). Examples 19 and 20 differ from the comparative examples by more than just glass fiber content; for instance, they have lower polyamide content than the comparative examples. See Spec. Table 4; see also Answer 22 (noting that Examples 19 and 20 comprise a “different amount of PA 6 2,4RV and PA 66 2,4RV”). Thus, Table 4 does not provide persuasive evidence that the compositions of claim 13 exhibit unexpected properties in comparison to compositions taught by Steenbakkers-Menting. 15 Appeal 2015-002326 Application 11/034,520 Appellants point to the Mercx Declaration as “an additional objective basis upon which it is reasonable to conclude that the claimed subject matter is unobvious.” Appeal Br. 9. Mr. Mercx expressed the belief that “one of skill in the art could not predict the properties of a resulting composition if, for example, the polyamide composition included between 35% and 60% by weight of filler.” Mercx Decl. 113; see also id. 117. However, this is contradicted by Steenbakkers-Menting’s teaching that the use of 10-40% glass fiber has advantages over the prior art, including “a V-0 rating according to UL 94,” and “good mechanical properties” as measured, for example by “ISO 527-1.” Steenbakkers-Menting 135. Mr. Mercx also testifies that during experimentation, the inventors “found that it was impossible to extrude a strand of a polyamide containing between 35% and 60% by weight of glass fibers and a flame retardant additive,” and that “it was practically impossible to extrude a flame-retardant composition containing compounds that contain glass fibers in amounts greater than 35% by weight.” Mercx Decl. 114—15. However, Mr. Mercx does not provide factual evidence to support these conclusions. See In re Brandstadter, 484 F.2d 1395, 1406 (CCPA 1973) (an affidavit fails in its purpose if it recites conclusions, but few facts to buttress those conclusions). In addition, Mr. Mercx does not provide evidence that people of ordinary skill in the art, other than the inventors, had access to experimental evidence leading to the expectation that extruding such compositions was impossible. Mr. Mercx also testifies that the claimed invention exhibits unexpected advantages, namely that increasing the rein forcing agent of the composition provides an unyielding electri cal performance of the compound while maintaining excellent mechanical properties and impact resistance. Based on my skill 16 Appeal 2015-002326 Application 11/034,520 and expertise in this field, it is my belief that this improved per formance, mechanical properties, and impact resistance is both unexpected and advantageous. It is also my belief that such ben efits cannot be derived from the teachings of the cited references. Id. ^ 18. However, these statements are not supported by experimental results in the Declaration, and to the extent that Mr. Mercx is referring to results set forth in the Specification, Appellants point only to Table 4, which, as discussed above, is insufficient evidence of unexpected results. Mr. Mercx further states that no prior art reference recognized or appreciated that a flame retardant polyamide composition containing between 35% and 60% of glass fiber filler could be mixed and extruded in a uniform strand. See id. Tffl 19—21. However, Appellants have not pointed to evidence that compositions within the full scope of claim 13 exhibit this allegedly unexpected property. See In re Harris, 409 F.3d 1339, 1343 (Fed. Cir. 2005) (Even assuming results are unexpected, applicant must show results covering the scope of the claimed range.) Moreover, we note that Steenbakkers-Menting teaches that the disclosed compositions may be molded and extruded. See Steenbakkers-Menting || 41 42.13 Having considered the appeal record as a whole, including Appellants’ evidence of unexpected results, we find that the preponderance of the evidence weighs most heavily in favor of the Examiner’s conclusion of obviousness.14 13 Appellants argue that the Examiner improperly discounted the testimony in the Mercx Declaration regarding extrudability because claim 13, itself, is not directed to extrudable strands. See Appeal Br. 9, 14; Reply Br. 5. Because the conclusion of obviousness of claim 13 does not depend on that determination, we decline to address it in our decision. 14 The Mercx Declaration also includes statements regarding other secondary considerations of obviousness, including commercial success, copying by 17 Appeal 2015-002326 Application 11/034,520 3. Examiner s New Grounds of Rejection Appellants argue that the Examiner improperly raised new issues in the Advisory Action, dated July 10, 2014, and in the Answer. Appeal Br. 14—15; Reply Br. 5—7. In particular, Appellants argue that the Examiner should have cited three additional references in the statement of the rejection: Olschewski,15 Machado,16 and Kilboume.17 Appeal Br. 14—15; Reply Br. 5—6 (citing In reHoch, 428 F.2d 1341, 1342 n.3 (CCPA 1970)). The Examiner cited these references to show that it was unsurprising in the art that “the use of glass fiber results in improved tensile strength.” Advisory Action 7—8; Answer 24. According to the Examiner, these references are merely evidentiary references cited in rebuttal to Appellants’ arguments of unexpected results, and are not cited as prior art. See Answer 24. However, because the Examiner did not explain in detail how the references are to be understood as rebutting Appellants’ evidence of unexpected results, see Advisory Action 7—8, we do not rely on the references in our analysis. Appellants also argue that the Examiner improperly raised in the Answer an “obvious to try” rationale for rejecting claim 13. Reply Br. 7 others, long felt need, and industry acquiescence. Mercx Decl. Tflf 24—31. Because Appellants do not raise these considerations in the Appeal Brief, we do not consider these arguments in our analysis. See 37 C.F.R. §§ 41.37(c)(l)(iv) (“[A]ny arguments or authorities not included in the appeal brief will be refused consideration by the Board for purposes of the present appeal.”). 15 Olschewski et al., U.S. Patent No. 4,339,374 (issued July 13, 1982). 16 Machado et al., U.S. Statutory Invention Reg. No. H1021 (published Feb. 4, 1992). 17 Kilboume, U.S. Patent No. 4,376,564 (issued Mar. 15, 1983). 18 Appeal 2015-002326 Application 11/034,520 (citing Answer 14). The question of whether or not the introduction of this rationale for the first time in the Answer was improper is a petitionable matter, and was waived because Appellants did not file a petition under 37 CFR § 1.181 (a) within two months from the mailing date of the Answer. See 37 CFR 41.40(a). Appellants argue that the Examiner’s “obvious to try” rationale is erroneous because there is no reasonable expectation of success of picking a com position out the myriad described by Steenbakkers[-Menting] that falls within the scope of the appealed claims and possesses the functional properties recited in the claims since evidence of record establishes that compositions within the scope of Steen- bakkers[-Menting] do not possess the claimed functional proper ties. Reply Br. 7. Significantly, Appellants do not direct us to any credible evidence demonstrating that the compositions disclosed in Steenbakkers- Menting falling within the scope of the claimed composition do not possess the claimed functional properties. As discussed above, a person of ordinary skill in the art, following the preferences taught by Steenbakkers-Menting, would have been led to a very small subset of compounds from among the larger genus described by the full disclosure. In addition, Steenbakkers- Menting teaches that success may be achieved by using a glass fiber composition in the range of at least 10-40%. See Steenbakkers-Menting 135. Therefore, Appellants’ argument does not persuade us that the 19 Appeal 2015-002326 Application 11/034,520 Examiner reversibly erred in rejecting claim 13, in part, on the ground the invention would have been “obvious to try.” For the above reasons, we are not persuaded that the Examiner reversibly erred in rejecting claim 13. Likewise, we are not persuaded of reversible error in the Examiner’s rejection of claims 15 and 17. DECISION The Examiner’s decision is affirmed. No time period for taking any subsequent action in connection with this appeal may be extended. See 37 C.F.R. § 1.136(a)(l)(iv) (2016). AFFIRMED 20 Copy with citationCopy as parenthetical citation