Ex Parte LEE et alDownload PDFPatent Trials and Appeals BoardMar 26, 201914410191 - (D) (P.T.A.B. Mar. 26, 2019) Copy Citation UNITED STA TES p A TENT AND TRADEMARK OFFICE APPLICATION NO. FILING DATE 14/410,191 12/22/2014 23373 7590 03/28/2019 SUGHRUE MION, PLLC 2100 PENNSYLVANIA A VENUE, N.W. SUITE 800 WASHINGTON, DC 20037 FIRST NAMED INVENTOR KunchanLEE UNITED STATES DEPARTMENT OF COMMERCE United States Patent and Trademark Office Address: COMMISSIONER FOR PATENTS P.O. Box 1450 Alexandria, Virginia 22313-1450 www .uspto.gov ATTORNEY DOCKET NO. CONFIRMATION NO. Q216443 1015 EXAMINER PARSONS, THOMAS H ART UNIT PAPER NUMBER 1729 NOTIFICATION DATE DELIVERY MODE 03/28/2019 ELECTRONIC Please find below and/or attached an Office communication concerning this application or proceeding. The time period for reply, if any, is set in the attached communication. Notice of the Office communication was sent electronically on above-indicated "Notification Date" to the following e-mail address(es): PPROCESSING@SUGHRUE.COM sughrue@sughrue.com USPTO@sughrue.com PTOL-90A (Rev. 04/07) UNITED STATES PATENT AND TRADEMARK OFFICE BEFORE THE PATENT TRIAL AND APPEAL BOARD Ex parte KUNCHAN LEE, YOSHINORI ABE, and YUJI ITO Appeal2018-004361 Application 14/410, 191 Technology Center 1700 Before JEFFREY B. ROBERTSON, DONNA M. PRAISS, and DEBRA L. DENNETT, Administrative Patent Judges. DENNETT, Administrative Patent Judge. DECISION ON APPEAL 1 STATEMENT OF THE CASE Appellant2 appeals under 35 U.S.C. § 134(a) from a rejection of claims 1-9. We have jurisdiction under 35 U.S.C. § 6(b ). We AFFIRM. 1 In our Decision, we refer to the Specification filed December 22, 2014 ("Spec."); the Final Office Action dated March 13, 2017 ("Final Act."); the Appeal Brief filed August 15, 2017 ("App. Br."); the Examiner's Answer dated January 25, 2018 ("Ans."); and the Reply Brief filed March 19, 2018 ("Reply Br."). 2 Appellant is the Applicant, SHOW A DENKO K.K., identified as the real party in interest. App. Br. 2. Appeal2018-004361 Application 14/410, 191 BACKGROUND The claims are directed to membrane electrode assemblies and fuel cells comprising the same. According to Applicant, in a direct methanol fuel cell (DMFC), a methanol crossover phenomenon occurs, such that methanol supplied to an anode permeates through the solid polymer electrolyte and reaches the cathode. Spec. ,r,r 3, 4. This methanol is oxidized by oxygen supplied to the cathode and is discharged as carbon dioxide. Id. ,r 4. In the oxidation reaction process, an oxidation reaction intermediate such as formic acid or formaldehyde is produced and discharged from the fuel cell. Id. Applicant sought to provide a fuel cell system in which the fuel cell's influence on system efficiency is small and only a small amount of oxidation reaction intermediate is discharged over a long period of time. Id. ,r 9. Claim 1, reproduced below from the Claims Appendix of the Appeal Brief, illustrates the claimed subject matter: 1. A membrane electrode assembly comprising an anode, a cathode and a solid polymer electrolyte membrane and having constitution in which the solid polymer electrolyte membrane is interposed between the anode and the cathode, wherein the cathode has a cathode catalyst layer and a cathode diffusion layer that is arranged on a surface of the cathode catalyst layer, said surface being on the opposite side to the solid polymer electrolyte membrane side, the cathode catalyst layer contains an oxygen reduction catalyst composed of composite particles each of which is constituted of a catalyst metal and a catalyst carrier, the catalyst metal contains palladium or a palladium alloy, the catalyst carrier contains, as constituent elements, 2 Appeal2018-004361 Application 14/410, 191 a transition metal element M 1 that is at least one selected from the group consisting of titanium, zirconium, niobium and tantalum, a transition metal element M2 other than the transition metal element M 1, carbon, nitrogen, and oxygen, the ratio of the number of atoms among the transition metal element Ml, the transition metal element M2, carbon, nitrogen and oxygen (transition metal element Ml :transition metal element M2:carbon:nitro- gen:oxygen) is (1-a):a:x:y:z (with the proviso that a, x, y and z are numbers ofO < a :S 0.5, 0 < x :S 7, 0 < y :S2 and 0 < z :S3), and the cathode diffusion layer contains an oxidation catalyst and a water-repellent resin. REFERENCES The Examiner relies on the following prior art in rejecting the claims on appeal: Suzuki et al. US 2011/0076591 Al ("Suzuki") Monden et al. US 2012/0070763 Al ("Monden") Toshiba Corp. 3 JP 2005-183014 ("JP 2005-183014") Mar. 31, 2011 Mar. 22, 2012 July 7, 2005 3 Appellant did not challenge the Examiner's use of a machine translation of Toshiba Corp. (cited in this Decision as JP 2005-183014), thus, have waived any objection to its evidentiary value. See In re Orbital Tech. Corp., 603 Fed. Appx. 924, 930 (Fed. Cir. 2015) (Appellant waived claims it might have had related to machine translation by pursuing appeal on that record.). 3 Appeal2018-004361 Application 14/410, 191 Monden et al. 4 ("Monden '334") WO 2009/104500 Al Aug. 27, 2009 REJECTIONS 5 The Examiner maintains and Appellant seeks review of the following rejections under 35 U.S.C. § I03(a): (1) claims 1--4, 6, and 9 over Suzuki in view of WO 2009/104500 Al; (2) claim 5 over Suzuki in view of WO 2009/104500 Al, and further in view of Monden; and (3) claims 7 and 8 over Suzuki in view of WO 2009/104500 Al, and further in view of JP 2005-183014. Final Act. 5-10; App. Br. 6.7 OPINION Appellant argues patentability of the claims as a group. See App. Br. 6-13. We select claim 1 as representative of the claims. 3 7 C.F .R. § 4I.37(c)(l)(iv). Claims 2-9 will stand or fall with claim 1. With respect to claim 1, the Examiner finds that Suzuki teaches the limitations of the claim except for the "constituent elements" of the catalyst carrier. Final Act. 5-7. The Examiner finds that WO 2009/104500 Al discloses the claimed catalyst constituent elements in the claimed ratios. Id. at 7. The Examiner determines that it would have been obvious to one of ordinary skill in the art at the time of the invention to modify Suzuki's membrane electrode assembly (MEA) with the catalyst carrier of 4 The Examiner used US 8,541,334 B2 as an English language equivalent of this reference. Citations in this Decision to WO 2009/104500 Al refer to figures and text in Monden '334. 5 Because this application claims an effective filing date before the March 16, 2013, effective date of the America Invents Act, we refer to the pre-AIA version of the statute. 4 Appeal2018-004361 Application 14/410, 191 WO 2009/104500 Al in order to provide a catalyst carrier having excellent heat resistance and high catalytic ability without increasing the specific surface area. Id. Appellant argues that Suzuki does not disclose a catalyst carrier containing, as constituent elements, a transition metal element, carbon, nitrogen, and oxygen. App. Br. 9. Appellant argues that WO 2009/104500 Al does not disclose a cathode diffusion layer containing an oxidation catalyst and a water-repellent resin. Id. Appellant argues that Monden, further cited by the Examiner in rejecting claim 5 (Final Act. 8-9), does not disclose a cathode diffusion layer containing an oxidation catalyst and a water-repellent resin. Id. at 10. Appellant argues that JP 2005-183014, further cited by the Examiner in rejecting claims 7 and 8 (Final Act. 9-10), does not disclose a catalyst carrier containing, as constituent elements, a transition metal element, carbon, nitrogen, and oxygen, or a cathode diffusion layer containing an oxidation catalyst and a water-repellent resin. Id. These arguments are unpersuasive of reversible error. Each of the above arguments addresses only individual references, and ignores the combination of references cited by the Examiner. One cannot show nonobviousness by attacking references individually when the rejection is based on a combination of references. In re Merck & Co., Inc., 800 F.2d 1091, 1097 (Fed. Cir. 1986). Each reference cited by the Examiner must be read, not in isolation, but for what it fairly teaches in combination with the prior art as a whole. See id. Appellant argues that none "of Suzuki, WO 2009/104500 Al, Monden, [or] JP-2005-183014 discloses or suggests that use of a specific 5 Appeal2018-004361 Application 14/410, 191 metal oxycarbonitride reduces emission of a reaction intermediate." App. Br. 11. Initially, we observe that claim 1 does not require the claimed membrane electrode assembly to reduce emission of a reaction intermediate. See App. Br. 15 (Claims App.). In re Van Geuns, 988 F.2d 1181, 1184 (Fed. Cir. 1993) ("[L ]imitations are not to be read into the claims from the specification."). Appellant contends that if Suzuki's fuel cell was modified to replace the carbon black catalyst carrier with WO 2009/104500 Al's metal oxycarbonitride, "it is presumed that a corresponding modified membrane electrode assembly would have properties regarding amount of an emitted reaction intermediate similar to those for the membrane electrode assembly in Suzuki." App. Br. 11. Appellant argues that, other than hindsight, there would have been no reason to expect the membrane electrode assembly of Suzuki as modified to have decreased the amount of an emitted reaction intermediate. Id. The skilled artisan "need not see the identical problem addressed in a prior art reference to be motivated to apply its teachings." Cross Med. Prods., Inc. v. Medtronic Sofamor Danek, Inc., 424 F.3d 1293, 1323 (Fed. Cir. 2005). The Supreme Court instructs us: "In determining whether the subject matter of a patent claim is obvious, neither the particular motivation nor the avowed purpose of the patentee controls. What matters is the objective reach of the claim. If the claim extends to what is obvious, it is invalid under § 103. . . . . The first error of the Court of Appeals in this case was ... holding that courts and patent examiners should look only to the problem the patentee was trying to solve." KSR Int 'l Co. v. Teleflex Inc., 550 U.S. 398, 419--20 (2007). "As long as some motivation or suggestion to combine the references is provided by the 6 Appeal2018-004361 Application 14/410, 191 prior art taken as a whole, the law does not require that the references be combined for the reasons contemplated by the inventors." In re Beattie, 974 F.2d 1309, 1312 (Fed. Cir. 1992). We are of the view that the Examiner's articulated rationale is sufficient to support the rejection. The Examiner finds that Suzuki and WO 2009/104500 Al are in a similar field of endeavor and are both concerned with catalyst carriers of membrane electrode assemblies, thus, it would have been obvious to modify Suzuki's catalyst carrier by incorporating the catalyst carrier of WO 2009/104500 Al to provide a catalyst carrier having excellent heat resistant that can exert high catalytic ability without increasing the specific surface area. Final Act. 7; Ans. 7. Where "a technique has been used to improve one device, and a person of ordinary skill in the art would recognize that it would improve similar devices in the same way, using the technique is obvious unless its actual application is beyond that person's skill." KSR, 550 U.S. at 401. "Express suggestion to substitute one equivalent for another need not be present to render such substitution obvious." In re Fout, 675 F.2d 297, 301 (CCPA 1982). Moreover, "[o ]bviousness does not require absolute predictability of success ... all that is required is a reasonable expectation of success." In re Kubin, 561 F.3d 1351, 1360 (Fed. Cir. 2009) (citing In re O'Farrell, 853 F.2d 894, 903---04 (Fed. Cir. 1988)). Thus, although the Examiner's rationale differs from Appellant's reasons for using a metal oxycarbonitride carrier, the Examiner has "articulated reasoning with some rational underpinning to support the legal conclusion of obviousness." In re Kahn, 441 F.3d 977, 988 (Fed. Cir. 2006). 7 Appeal2018-004361 Application 14/410, 191 Appellant's contention that the rejection is based on mere hindsight is unpersuasive. Appellant argues that the combination of the claimed cathode catalyst layer and the claimed cathode diffusion layer in the MEA provides unexpected superior results, making the claim nonobvious over the references. App. Br. 8. Appellant argues that the fuel cells in Examples 1 to 3 of the Specification discharged only 1/10 to 1/30 of the reaction intermediates (formaldehyde, formic acid, and methyl formate) that were discharged by the fuel cell of Comparative Example 1. Id. Appellant contends that Comparative Example 1, employing platinum-supported carbon black to form the cathode catalyst layer, corresponds to the MEA taught by Suzuki. Id. at 12. Appellant argues, therefore, that both the claimed cathode catalyst layer (not present in Suzuki) and the claimed cathode diffusion layer ( disclosed in Suzuki) are required to achieve considerable reduction of reaction intermediates. Id. at 8. "[T]he burden of showing unexpected results rests on he who asserts them." In re Klosak, 455 F.2d 1077, 1080 (CCPA 1972). When used as evidence of nonobviousness, unexpected results must be shown to be unexpected compared with the closest prior art. In re Baxter Travenol Labs., 952 F.2d 388, 392 (Fed. Cir. 1991). Superiority alone is not sufficient to show that the result is unexpected. Pfizer, Inc. v. Apotex, Inc., 480 F.3d 1348, 13 71 (Fed. Cir. 2007) ("[ A ]ny superior property must be unexpected to be considered as evidence of non-obviousness." (emphasis in original)). Appellant provides data on the amounts of formaldehyde, formic acid, and methyl formate discharged by fuel cells comprising either 5 wt% Pd- supported TiFeCNO ( catalyst 1) or 5 mass% Pt-supported carbon black 8 Appeal2018-004361 Application 14/410, 191 (catalyst 5). Spec. ,r,r 243-267, 276-282. The data shows improvement in results obtained with one catalyst versus the other, but Appellant provides only attorney argument that the results obtained with catalyst 5 would have been unexpected by one of ordinary skill in the art at the time of the invention. It is well settled that arguments of counsel cannot take the place of factually supported objective evidence. See, e.g., In re Huang, I 00 F .3d 135, 139--40 (Fed. Cir. 1996); In re De Blauwe, 736 F.2d 699, 705 (Fed. Cir. 1984). Of greater importance, Appellant's evidence is not commensurate with the scope of claim 1. In re Harris, 409 F.3d 1339, 1344 (Fed. Cir. 2005) (unexpected results must be "commensurate in scope with the degree of protection sought by the claim[ s ]" on appeal). Claim 1 encompasses catalyst carriers containing, inter alia, "a transition metal element Ml that is at least one selected from the group consisting of titanium, zirconium, niobium and tantalum," and "a transition metal element M2 other than the transition metal element Ml." App. Br. 15 (Claims App.). The data provided, however, is limited to a single catalyst carrier containing Tio.91Feo.09C2.70No.070uo. Spec. ,r 241. Thus, data is available for only a single amount of only one of the transition metals designated as transition metal element Ml, only a single amount of a single transition metal M2 that can be any transitional metal other than those specified as Ml, and only single amounts of carbon, nitrogen, and oxygen. See id. Claim 1 is substantially broader in scope than the limited data available, even assuming it supports unexpected results. Such evidence is insufficient to overcome the Examiner's prima facie case of obviousness. 9 Appeal2018-004361 Application 14/410, 191 We are not persuaded by Appellant's argument that, because "all of titanium, zirconium, niobium and tantalum are metals falling in periodic table Group 4 or Group 5," they have "similar features in common," and one of ordinary skill in the art would have expected the same superior effects provided with Pd-supported TiFeCNO when titanium is substituted with zirconium, niobium or tantalum. Reply Br. 4. Counsel's argument "cannot take the place of evidence lacking in the record." Estee Lauder Inc. v. L 'Orea!, S.A., 129 F.3d 588, 595 (Fed. Cir. 1997). Appellant's arguments fail to identify any reversible error in the Examiner's rejection. In re Jung, 637 F.3d 1356, 1365 (Fed. Cir. 2011). We sustain the rejection of claim 1 as obvious over Suzuki in view of WO 2009/104500 Al. For the same reasons, we sustain the rejections of claims 2-9, which Appellant did not argue separately. DECISION The rejections of claims 1-9 are affirmed. No time period for taking any subsequent action in connection with this appeal may be extended under 37 C.F.R. § 1.136(a)(l )(iv). AFFIRMED 10 Copy with citationCopy as parenthetical citation