Ex Parte Gull¿ et alDownload PDFPatent Trial and Appeal BoardSep 6, 201613005651 (P.T.A.B. Sep. 6, 2016) Copy Citation UNITED STA TES p A TENT AND TRADEMARK OFFICE APPLICATION NO. FILING DATE FIRST NAMED INVENTOR 13/005,651 01/13/2011 Andrea F. Gulll 20311 7590 09/08/2016 LUCAS & MERCANTI, LLP 30 BROAD STREET 21st FLOOR NEW YORK, NY 10004 UNITED STATES DEPARTMENT OF COMMERCE United States Patent and Trademark Office Address: COMMISSIONER FOR PATENTS P.O. Box 1450 Alexandria, Virginia 22313-1450 www .uspto.gov ATTORNEY DOCKET NO. CONFIRMATION NO. 267-127 2981 EXAMINER FRIDAY, STEVEN A ART UNIT PAPER NUMBER 1756 NOTIFICATION DATE DELIVERY MODE 09/08/2016 ELECTRONIC Please find below and/or attached an Office communication concerning this application or proceeding. The time period for reply, if any, is set in the attached communication. Notice of the Office communication was sent electronically on above-indicated "Notification Date" to the following e-mail address( es): info@lmiplaw.com PTOL-90A (Rev. 04/07) UNITED STATES PATENT AND TRADEMARK OFFICE BEFORE THE PATENT TRIAL AND APPEAL BOARD Ex parte ANDREA F. GULLA and MARIACHIARA BENEDETTO Appeal2015-004429 Application 13/005,651 Technology Center 1700 Before JEFFREY T. SMITH, KAREN M. HASTINGS, and MICHAEL P. COLAIANNI, Administrative Patent Judges. HASTINGS, Administrative Patent Judge. DECISION ON APPEAL STATEMENT OF THE CASE Appellants seek our review under 35 U.S.C. § 134(a) of the Examiner's decision rejecting claims 14--19 and 21-25. We have jurisdiction over the appeal under 35 U.S.C. § 6(b ). We AFFIRM. Appeal2015-004429 Application 13/005,651 Independent claims 14 and 21 read (emphasis added to highlight disputed limitations): 14. Process of abatement of the Total Organic Content in an aqueous solution containing one or more organic species, said one or more organic species having at least one carbon atom involved in a conjugated unsaturated bond, optionally aromatic, said carbon atom having an electron-attracting substituent, the process comprising the steps of: subjecting the aqueous solution to a reduction treatment at the cathode of a first electrochemical cell; and thereafter subjecting the treated aqueous solution to an electrochemical oxidation treatment, wherein said reduction step is carried out at a current density lower than 1 kA/m2 and said oxidation step is carried out at current density comprised between 1 and 3 kA/m2. 21. Process of abatement of the Total Organic Content in an aqueous solution containing one or more organic species, said one or more organic species having at least one carbon atom involved in a conjugated unsaturated bond, optionally aromatic, said carbon atom having an electron-attracting substituent, the process comprising the steps of subjecting the aqueous solution to: a reduction treatment at the cathode of an undivided cell to obtain a pre-reduced organic species; and a simultaneous oxidation treatment of said pre-reduced organic species at the anode of said undivided cell, wherein said reduction step and simultaneous oxidation step is carried out at a current density lower than 1 kA/m2. The Examiner maintains the following rejections: (a) claims 14, 16 and 18 rejected under 35 U.S.C. § 103(a) as unpatentable over Cong (Cong, Y., Wu, Z., Tan, T. "Dechlorination by 2 Appeal2015-004429 Application 13/005,651 combined electrochemical reduction and oxidation." May 2005. Journal of Zhejiang University SCIENCE B. Vol. 6, Issue 6. pp. 563-568) and Comninellis (Comninellis, Ch. and Nerini, A. "Anodic oxidation of phenol in the presence of NaCl for wastewater treatment" Journal of Applied Electrochemistry. Jan. 1995. Volume 25, Issue 1. pp. 23-28), (b) claims 21, 22, and 24 rejected under 35 U.S.C. § 103(a) as unpatentable over Cong and Van Duin (US 4,443,309, issued April 17, 1984), (c) claims 15 and 17 rejected under 35 U.S.C. § 103(a) as unpatentable over Cong, Comninellis and Moeglich (US 4, 131,526, issued December 26, 1978), (d) claim 19 rejected under 35 U.S.C. § 103(a) as unpatentable over Cong, Comninellis and Rajeshwar (Rajeshwar, K., Ibanez, J. Environmental Electrochemistry: Fundamentals and Applications in Pollution Abatement. 1997 (no month). Academic Press, Inc. pp. 363-378), (e) claim 23 rejected under 35 U.S.C. § 103(a) as unpatentable over Cong, Van Duin and Rideout (US 4,260,463, issued April 7, 1981), and (f) claim 25 rejected under 35 U.S.C. § 103(a) as unpatentable over Cong, Van Duin and Rajeshwar. For Rejection (a), Appellants do not argue any claim separate from the other. See Appeal Brief, generally. For Rejection (b ), Appellants present arguments for independent claim 21 but do not present separate arguments for dependent claims 22 and 24. Id. In addressing Rejections (c}-(t), Appellants rely on the arguments presented when discussing the independent claims 14 and 21, and do not address or further distinguish the additionally cited secondary references based on the additional limitations of the respectively rejected claims. Accordingly, we select independent claims 14 and 21 as representative of the claimed subject matter before us on appeal 3 Appeal2015-004429 Application 13/005,651 for the respective Rejections (a) and (b). Claims 15-19 and 22-25 stand or fall with their respective independent claim. ANALYSIS We have thoroughly reviewed each of Appellants' arguments for patentability. However, we determine that a preponderance of the evidence supports the Examiner's § 103 rejections of representative independent claims 14 and 21. Accordingly, we will sustain all of the Examiner's rejections for essentially those reasons expressed in the Answer and we add the following for emphasis. Rejection (a) Independent claim 14 requires sequential reduction and oxidation treatment of an aqueous solution containing one or more organic species where the oxidation treatment is carried out at current density comprised between 1 and 3 kA/m2. The Examiner found Cong discloses a process of abatement of the hazardous organic material chlorophenol from wastewater comprising reduction of chlorophenol to phenol and subsequent oxidation of phenol to low toxicity organic acids and/or C02 and H20. Final Act. 3; Cong 563- 565, 567. The Examiner found Cong does not teach that the oxidation step is carried out at a current density of between 1 and 3 kA/m2 as required by the subject matter of claim 14. Final Act. 4. The Examiner found Comninellis teaches a process of removing phenol from wastewater through anodic oxidation of phenol at a current density range of 0.5-3 kA/m2, which 4 Appeal2015-004429 Application 13/005,651 overlaps the current density range for the claimed oxidation step. 1 Final Act. 4; Cong Abstract; Comninellis Abstract, 24, 26. The Examiner determined it would have been obvious to a person of ordinary skill in the art to modify the process taught by Cong by applying the oxidation current density range of Comninellis to Cong's oxidation step because Comninellis describes it as technically reasonable for oxidation of phenols. Final Act. 4; Comninellis 26. Appellants principally argue Comninellis does not disclose a reduction step before oxidation, the problem with electrode fouling associated with oxidation of the species to be abated before reduction is completed, or suggests the combination of reduction and oxidation at a specific current density play any role in the treatment of wastewater. App. Br. 5. Thus, Appellants argue, absent impermissible hindsight, the disclosure of Comninellis would discourage one skilled in the art from an approach involving the inclusion of the oxidation step at Comninellis' described current density because Comninellis provides no discussion of such combination of reduction and oxidation. App. Br. 6. We are unpersuaded by these arguments. As noted by the Examiner, Cong was relied upon to teach the combined use of the reduction and oxidation steps and Comninellis was cited to teach that it was known to operate the oxidation step of phenol at the claimed current density levels. Ans. 10. Appellants' arguments do not address the Examiner's reasons for combining the teachings of the cited art. It is well established that 1 We note that Appellants do not dispute the Examiners finding that Comninellis' current density of 0.05-3 A/cm2, as described in page 24, equals 0.5-3 kA/m2. 5 Appeal2015-004429 Application 13/005,651 nonobviousness cannot be established by attacking the references individually when the rejection is predicated upon a combination of prior art disclosures. In re Merck & Co., 800 F.2d 1091, 1097 (Fed. Cir. 1986); In re Keller, 642 F.2d 413, 425-26 (CCPA 1981) ("The test for obviousness ... is what the combined teachings of the references would have suggested to those of ordinary skill in the art."). Thus, Appellants' arguments do not point to reversible error in the Examiner's determination of obviousness. While Appellants argue the process taught by Cong is impractical from an industrial standpoint because the current density for the reduction step of 0.012 kA/m2 is low, the Examiner aptly points out that Appellants' claimed reduction step at a current density lower than 1 kA/m2 encompasses Cong's disclosed reduction step. App. Br. 5; Ans. 9. Thus, Appellants have not adequately distinguished the claimed reduction step from the one taught by Cong. Appellants further argue Examples 1-3 and Comparative Examples 1 and 2 in the Specification demonstrate surprising results when the reduction step is carried at a current density not higher than 1 kA/m2 because no fouling of the anodic surface was observed and the total content of carbon was significantly lower than the content detected in the original waste. App. Br. 7-8. We are also unpersuaded by this evidence. Appellants' Examples 1-3 conduct the reduction step only at a current density of 0.6 kA/m2. Appellants have not adequately explained why this single current density is representative of the entire scope of current densities encompassed by the claimed range of lower than 1 kA/m2 recited in claim 14. That is, Appellants' showing is not commensurate in scope with the subject matter of 6 Appeal2015-004429 Application 13/005,651 claim 14. In addition, as noted by the Examiner, Appellants' proferred showing in not against the closest prior art, Cong in this case. Ans. 11-12. Accordingly, we affirm the Examiner's prior art rejections of claims 14--19 under 35 U.S.C. § 103(a) (Rejections (a), (c) and (d)) for the reasons presented by the Examiner and given above. Rejection (b) Independent claim 21 requires that the reduction and oxidation steps be conducted simultaneously at a current density lower than 1 kA/m2. We refer to the Examiner's Final Action for a statement of the rejection. Final Act. 7-8. Appellants principally argue that one of ordinary skill in the art reading Cong in its entirety would be led to believe that electrochemical reduction followed by electrochemical oxidation is an effective and feasible method and, absent impermissible hindsight, there would have been no motivation to use Van Duin's simultaneous technique. App. Br. 10. Appellants further argue Cong does not require the presence of micelle- forming material and also does not provide guidance as to the current density applied to the disclosed oxidation step while Van Duin's method is carried out with lower energy consumption due to the presence of micelle- forming material. App. Br. 10-11. Thus, according to Appellants, there is no clear guidance to determine if it is feasible to operate Cong's method of abatement using Van Duin's simultaneous reduction/oxidation technique to obtain predictable results. Id. We are unpersuaded by Appellants' arguments. The Examiner found Cong discloses a process to abate chlorophenol (halogenated hydrocarbon) 7 Appeal2015-004429 Application 13/005,651 from wastewater comprising subjecting the wastewater to an electrochemical reduction treatment and subsequently to an oxidation treatment where at least the reduction treatment is carried out at a current density lower than 1 kA/m2. Final Act. 7-8; Cong 563-565, 567. The Examiner found Van Duin teaches the use of simultaneous electrochemical reduction/ oxidation to treat toxic chemical wastes including halogenated hydrocarbons as a known technique for abatement of halogenated hydrocarbons. Final Act. 8; Van Duin Abstract, col. 4, 11. 6-11. In fact, Van Duin teaches the use of divided and undivided cells as known techniques for abatement of halogenated hydrocarbons. Van Duin Examples 1--4. Thus, the Examiner provided a reasonable basis why one skilled in the art would have modified the abatement process of Cong by using the undivided cell taught by Van Duin so as to allow simultaneous reduction/oxidation treatment of the wastewater. Final Act. 8. That is, the Examiner determined that one of ordinary skill in the art would have been led to the known technique of Van Duin with the reasonable expectation of successfully abating halogenated hydrocarbons from wastewater. See KSR Int'! Co. v. Teleflex, Inc., 550 U.S. 398, 416 (2007) ("[W]hen a patent claims a structure [or method] already known in the prior art that is altered by the mere substitution of one element [or step] for another known in the field, the combination must do more than yield a predictable result." (citing United States v. Adams, 383 U.S. 39, 50-51 (1966)); In re Fout, 675 F.2d 297, 301 (CCPA 1982) ("Express suggestion to substitute one equivalent for another need not be present to render such substitution obvious."); In re Mayne, 104 F.3d 1339, 1340 (Fed. Cir. 1997) ("Because the applicants merely substituted one element known in the art for a known equivalent, this court affirms [the rejection for obviousness]."). 8 Appeal2015-004429 Application 13/005,651 Thus, on this record, Appellants have not adequately explained why one skilled in the art would not have been capable of adapting the method of Cong to use Van Duin' s simultaneous reduction/ oxidation treatment for Cong's process of wastewater treatment. While Appellants argue Van Duin' s method of abatement carries out the electrolysis in the presence of a micelle-forming material, we note the claim is written using the open transitional language "comprising" and, thus, does not exclude the use micelle-forming material as part of the abatement process. App. Br. 10; Van Duin Examples 3, 4, col. 1, 11. 30-35. Accordingly, we affirm the Examiner's prior art rejections of claims 21-25 under 35 U.S.C. § 103(a) (Rejections (b), (e) and (f)) for the reasons presented by the Examiner and given above. ORDER The Examiner's prior art rejections of claims 14--19 and 21-25 are affirmed. TIME PERIOD No time period for taking any subsequent action in connection with this appeal may be extended under 37 C.F.R. § 1.136(a)(l). AFFIRMED 9 Copy with citationCopy as parenthetical citation